TY - JOUR
T1 - Anomalous Nernst effect in a microfabricated thermoelectric element made of chiral antiferromagnet Mn3Sn
AU - Narita, Hideki
AU - Ikhlas, Muhammad
AU - Kimata, Motoi
AU - Nugroho, Agustinus Agung
AU - Nakatsuji, Satoru
AU - Otani, Yoshichika
N1 - Funding Information:
This work was partially supported by JST CREST (Grant No. JPMJCR15Q5) from JST and Grants-in-Aid for Scientific Research on Innovative Areas (26103002 and 15H05883) of the Ministry of Education, Culture, Sports, Science, and Technology of Japan. H.N. is grateful to E. Saitoh and T. Kikkawa of Tohoku University for hosting him during an internship supported by Grants-in-Aid for Scientific Research on Innovative Areas (26103001). Also, we are grateful to Y. Omori and T. Higo from the Institute for Solid State Physics, University of Tokyo, for fruitful discussions.
Publisher Copyright:
© 2017 Author(s).
PY - 2017/11/13
Y1 - 2017/11/13
N2 - Toward realizing a thermopile made of the chiral anti-ferromagnet Mn3Sn, focused ion beam (FIB) lithography was employed to microfabricate a thermoelectric element consisting of a Ta/Al2O3/Mn3Sn layered structure. In this device, the Ta layer acts as a heater producing Joule heat diffusing across the Al2O3 insulating layer into the thin Mn3Sn layer. The measured Nernst signal exhibits a clear hysteresis in an applied temperature gradient and magnetic field at 300 K, and its magnitude is proportional to the square of the electrical current applied to the Ta heater. The spontaneous, zero field voltage signal in the device is of the order of a few μV, which is almost the same order of magnitude as observed in the bulk single-crystal Mn3Sn under a temperature gradient. The anomalous Nernst coefficient SANE of the microfabricated element was determined using a temperature gradient simulated by finite-element modeling. The obtained value of SANE is 0.27 μV/K, which is in good agreement with that of the reported experimental value of SANE (0.3 μV/K) for bulk single-crystal Mn3Sn. This result indicates that FIB microfabrication does not significantly alter the thermoelectric properties of bulk Mn3Sn. As the chiral antiferromagnet produces almost no stray field, our study opens the avenue for the fabrication of an efficient thermopile by densely packing the microfabricated antiferromagnetic elements.
AB - Toward realizing a thermopile made of the chiral anti-ferromagnet Mn3Sn, focused ion beam (FIB) lithography was employed to microfabricate a thermoelectric element consisting of a Ta/Al2O3/Mn3Sn layered structure. In this device, the Ta layer acts as a heater producing Joule heat diffusing across the Al2O3 insulating layer into the thin Mn3Sn layer. The measured Nernst signal exhibits a clear hysteresis in an applied temperature gradient and magnetic field at 300 K, and its magnitude is proportional to the square of the electrical current applied to the Ta heater. The spontaneous, zero field voltage signal in the device is of the order of a few μV, which is almost the same order of magnitude as observed in the bulk single-crystal Mn3Sn under a temperature gradient. The anomalous Nernst coefficient SANE of the microfabricated element was determined using a temperature gradient simulated by finite-element modeling. The obtained value of SANE is 0.27 μV/K, which is in good agreement with that of the reported experimental value of SANE (0.3 μV/K) for bulk single-crystal Mn3Sn. This result indicates that FIB microfabrication does not significantly alter the thermoelectric properties of bulk Mn3Sn. As the chiral antiferromagnet produces almost no stray field, our study opens the avenue for the fabrication of an efficient thermopile by densely packing the microfabricated antiferromagnetic elements.
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U2 - 10.1063/1.5000815
DO - 10.1063/1.5000815
M3 - Article
AN - SCOPUS:85034032130
SN - 0003-6951
VL - 111
JO - Applied Physics Letters
JF - Applied Physics Letters
IS - 20
M1 - 202404
ER -