TY - JOUR
T1 - Collective and local excitations in Ba2 CoTeO6
T2 - A composite system of a spin-1/2 triangular-lattice Heisenberg antiferromagnet and a honeycomb-lattice J1-J2 Ising antiferromagnet
AU - Chanlert, Purintorn
AU - Kurita, Nobuyuki
AU - Tanaka, Hidekazu
AU - Kimata, Motoi
AU - Nojiri, Hiroyuki
N1 - Publisher Copyright:
© 2017 American Physical Society.
PY - 2017/8/15
Y1 - 2017/8/15
N2 - We report the results of multifrequency high-magnetic-field electron-spin resonance (ESR) measurements on the highly frustrated antiferromagnet Ba2CoTeO6. This compound is magnetically composed of two subsystems A and B, which are described as a spin-1/2 triangular-lattice Heisenberg antiferromagnet and a honeycomb-lattice J1-J2 Ising antiferromagnet, respectively. Ba2CoTeO6 undergoes successive magnetic phase transitions at TN1=12.0 K and TN2=3.0 K. For a magnetic field H parallel to the c axis, subsystem B exhibits successive metamagnetic transitions with magnetization plateaus at one-third and one-half of the saturation magnetization. Below TN2, we observed collective ESR modes for Hc, which are characteristic of a triangular-lattice Heisenberg antiferromagnet with weak easy-plane anisotropy. We also observed a local excitation mode, which can be assigned as a single flip of the Ising-like spin of subsystem B. From a detailed analysis of the collective and local ESR modes, combined with the magnetization process, we determined the magnetic parameters of subsystems A and B, and confirmed that the two subsystems are almost decoupled.
AB - We report the results of multifrequency high-magnetic-field electron-spin resonance (ESR) measurements on the highly frustrated antiferromagnet Ba2CoTeO6. This compound is magnetically composed of two subsystems A and B, which are described as a spin-1/2 triangular-lattice Heisenberg antiferromagnet and a honeycomb-lattice J1-J2 Ising antiferromagnet, respectively. Ba2CoTeO6 undergoes successive magnetic phase transitions at TN1=12.0 K and TN2=3.0 K. For a magnetic field H parallel to the c axis, subsystem B exhibits successive metamagnetic transitions with magnetization plateaus at one-third and one-half of the saturation magnetization. Below TN2, we observed collective ESR modes for Hc, which are characteristic of a triangular-lattice Heisenberg antiferromagnet with weak easy-plane anisotropy. We also observed a local excitation mode, which can be assigned as a single flip of the Ising-like spin of subsystem B. From a detailed analysis of the collective and local ESR modes, combined with the magnetization process, we determined the magnetic parameters of subsystems A and B, and confirmed that the two subsystems are almost decoupled.
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U2 - 10.1103/PhysRevB.96.064419
DO - 10.1103/PhysRevB.96.064419
M3 - Article
AN - SCOPUS:85028709247
SN - 2469-9950
VL - 96
JO - Physical Review B
JF - Physical Review B
IS - 6
M1 - 064419
ER -