Effective staggered field for strongly anisotropic moments on the low-symmetry site in Ce2Pd2Pb

N. Kabeya, R. Kogane, S. Takahara, S. Nakamura, K. Araki, K. Katoh, N. Kimura, A. Ochiai

Research output: Contribution to journalArticlepeer-review

Abstract

We studied magnetic-field responses of a low-symmetrical site, i.e., an orthorhombic site in a tetragonal crystal, in Ce2Pd2Pb, which exhibits a strong axial moment in the cerium site. Considering two orthogonalized local-coordinate systems on the cerium site, the field responses of the moment can be expressed as a product of the external field and spatial variation of the g factor and be regarded as the responses of an effective staggered field for the isotropic pseudospin sp=1/2 state. We obtained H-T phase diagrams of Ce2Pd2Pb under the fields H(100) and H(110) from thermodynamic measurements and identified magnetization plateaus for several phases. Assuming the effective staggered field, we can explain the specific heat of Ce2Pd2Pb under high fields. The result indicates that a partially ordered state in which one-half of the total cerium moments contributes to the long-range order is realized for H(110), where the staggered component becomes maximum. Furthermore, a slight incline of the field results in a change in the ordering nature of the partially ordered phase, demonstrating the controllability of the effective staggered field.

Original languageEnglish
Article number174421
JournalPhysical Review B
Volume110
Issue number17
DOIs
Publication statusPublished - 2024 Nov 1

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