Magnetic behavior of cosputtered Fe-Zr amorphous thin films exhibiting perpendicular magnetic anisotropy

Parmanand Sharma, Hisamichi Kimura, Akihisa Inoue

Research output: Contribution to journalArticlepeer-review

28 Citations (Scopus)


Excellent mechanical properties of amorphous or glassy metals along with the capability to fabricate sub-50-nm patterns promise their application as a futuristic material for production of various nano- or microelectromechanical systems. In addition to their applications, these materials pose a lot of challenges in understanding their fundamental properties because of their random structure and involvement of three or more different kinds of atoms. The amorphous Fe-Zr system which is reported to exhibit superconductivity, ferromagnetism, spin glass, and antiferromagnetism is an ideal system to understand. The controversial magnetic properties of this system are still a subject of debate. In the present paper we revisited Fe-Zr system and studied their detailed magnetic properties in the temperature range of 5-330 K. Fex Zr100-x (x=63, 68, 76, 86, 92, and 93 at.%) thin films were deposited on silicon (100) substrate by a cosputtering technique. The Curie temperature (Tc) is shown to increase almost linearly with an increase in Fe concentration, but it decreases rapidly for the Fe-rich films. The films with x up to ∼86 at.% have a strange shape of the hysteresis loop and are shown to exhibit perpendicular magnetic anisotropy with a stripe domain structure. Hysteresis loop shapes are correlated with the magnetic structure of the films, and provide an easy understanding of magnetic properties. It has been shown that the Fe-rich films are composed of antiferromagnetic Fe clusters which are embedded in the ferromagnetic amorphous FeZr.

Original languageEnglish
Article number134414
JournalPhysical Review B - Condensed Matter and Materials Physics
Issue number13
Publication statusPublished - 2008 Oct 17


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