TY - JOUR
T1 - Magnetization process and collective excitations in the s=1/2 triangular-lattice heisenberg antiferromagnet Ba3CoSb 2O9
AU - Susuki, Takuya
AU - Kurita, Nobuyuki
AU - Tanaka, Takuya
AU - Nojiri, Hiroyuki
AU - Matsuo, Akira
AU - Kindo, Koichi
AU - Tanaka, Hidekazu
PY - 2013/6/24
Y1 - 2013/6/24
N2 - We have performed high-field magnetization and electronic spin resonance (ESR) measurements on Ba3CoSb2O9 single crystals, which approximates the two-dimensional (2D) S=1/2 triangular-lattice Heisenberg antiferromagnet. For an applied magnetic field H parallel to the ab plane, the entire magnetization curve including the plateau at one-third of the saturation magnetization (Ms) is in excellent agreement with the results of theoretical calculations except a small step anomaly near (3/5)M s, indicative of a theoretically undiscovered quantum phase transition. However, for Hâ̂¥c, the magnetization curve exhibits a cusp near Ms/3 owing to the weak easy-plane anisotropy and the 2D quantum fluctuation. From a detailed analysis of the collective ESR modes observed in the ordered state, combined with the magnetization process, we have determined all the magnetic parameters including the interlayer and anisotropic exchange interactions.
AB - We have performed high-field magnetization and electronic spin resonance (ESR) measurements on Ba3CoSb2O9 single crystals, which approximates the two-dimensional (2D) S=1/2 triangular-lattice Heisenberg antiferromagnet. For an applied magnetic field H parallel to the ab plane, the entire magnetization curve including the plateau at one-third of the saturation magnetization (Ms) is in excellent agreement with the results of theoretical calculations except a small step anomaly near (3/5)M s, indicative of a theoretically undiscovered quantum phase transition. However, for Hâ̂¥c, the magnetization curve exhibits a cusp near Ms/3 owing to the weak easy-plane anisotropy and the 2D quantum fluctuation. From a detailed analysis of the collective ESR modes observed in the ordered state, combined with the magnetization process, we have determined all the magnetic parameters including the interlayer and anisotropic exchange interactions.
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U2 - 10.1103/PhysRevLett.110.267201
DO - 10.1103/PhysRevLett.110.267201
M3 - Article
AN - SCOPUS:84879474409
SN - 0031-9007
VL - 110
JO - Physical Review Letters
JF - Physical Review Letters
IS - 26
M1 - 267201
ER -