Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

Yukiyoshi Ohtsuki; Kazuyuki Nakagami; Yuichi Fujimura; Wusheng Zhu; Herschel Rabitz

doi:10.1063/1.1368133

Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

Yukiyoshi Ohtsuki, Kazuyuki Nakagami, Yuichi Fujimura, Wusheng Zhu, Herschel Rabitz

SCI - Chemistry

Research output: Contribution to journal › Article › peer-review

61 Citations (Scopus)

Abstract

A new efficient algorithm was proposed for solving coupled quantum control equations allowing multiple target operators with desired expected values to specify an objective state. To design a field that transferred a molecule to an objective state an optimal control procedure was presented. Constraints on the time behavior of specified operators during the control period were taken into account. The algorithm represented in the quadruple-space notation reduced to double-space notation in the absence of time-dependant constraints.

Original language	English
Pages (from-to)	8867-8876
Number of pages	10
Journal	Journal of Chemical Physics
Volume	114
Issue number	20
DOIs	https://doi.org/10.1063/1.1368133
Publication status	Published - 2001 May 22

ASJC Scopus subject areas

Physics and Astronomy(all)
Physical and Theoretical Chemistry

Access to Document

10.1063/1.1368133

Cite this

Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control. / Ohtsuki, Yukiyoshi; Nakagami, Kazuyuki; Fujimura, Yuichi et al.
In: Journal of Chemical Physics, Vol. 114, No. 20, 22.05.2001, p. 8867-8876.

Research output: Contribution to journal › Article › peer-review

@article{73fe9d43fdaa4a3bab018cd4e699f19d,

title = "Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control",

abstract = "A new efficient algorithm was proposed for solving coupled quantum control equations allowing multiple target operators with desired expected values to specify an objective state. To design a field that transferred a molecule to an objective state an optimal control procedure was presented. Constraints on the time behavior of specified operators during the control period were taken into account. The algorithm represented in the quadruple-space notation reduced to double-space notation in the absence of time-dependant constraints.",

author = "Yukiyoshi Ohtsuki and Kazuyuki Nakagami and Yuichi Fujimura and Wusheng Zhu and Herschel Rabitz",

year = "2001",

month = may,

day = "22",

doi = "10.1063/1.1368133",

language = "English",

volume = "114",

pages = "8867--8876",

journal = "Journal of Chemical Physics",

issn = "0021-9606",

publisher = "American Institute of Physics Publising LLC",

number = "20",

}

TY - JOUR

T1 - Quantum optimal control of multiple targets

T2 - Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

AU - Ohtsuki, Yukiyoshi

AU - Nakagami, Kazuyuki

AU - Fujimura, Yuichi

AU - Zhu, Wusheng

AU - Rabitz, Herschel

PY - 2001/5/22

Y1 - 2001/5/22

N2 - A new efficient algorithm was proposed for solving coupled quantum control equations allowing multiple target operators with desired expected values to specify an objective state. To design a field that transferred a molecule to an objective state an optimal control procedure was presented. Constraints on the time behavior of specified operators during the control period were taken into account. The algorithm represented in the quadruple-space notation reduced to double-space notation in the absence of time-dependant constraints.

AB - A new efficient algorithm was proposed for solving coupled quantum control equations allowing multiple target operators with desired expected values to specify an objective state. To design a field that transferred a molecule to an objective state an optimal control procedure was presented. Constraints on the time behavior of specified operators during the control period were taken into account. The algorithm represented in the quadruple-space notation reduced to double-space notation in the absence of time-dependant constraints.

UR - http://www.scopus.com/inward/record.url?scp=0035932859&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=0035932859&partnerID=8YFLogxK

U2 - 10.1063/1.1368133

DO - 10.1063/1.1368133

M3 - Article

AN - SCOPUS:0035932859

SN - 0021-9606

VL - 114

SP - 8867

EP - 8876

JO - Journal of Chemical Physics

JF - Journal of Chemical Physics

IS - 20

ER -

Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

Abstract

ASJC Scopus subject areas

Access to Document

Other files and links

Fingerprint

Cite this