TY - JOUR
T1 - Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
AU - Yukawa, R.
AU - Kobayashi, M.
AU - Kanda, T.
AU - Shiga, D.
AU - Yoshimatsu, K.
AU - Ishibashi, S.
AU - Minohara, M.
AU - Kitamura, M.
AU - Horiba, K.
AU - Santander-Syro, A. F.
AU - Kumigashira, H.
N1 - Funding Information:
is supported by public grants from the Centre National de la Recherche Scientifique (CNRS), International Research Project (IRP) EXCELSIOR, and the French National Research Agency (ANR), project Fermi-NESt No. ANR-16-CE92-0018. The work performed at KEK-PF was approved by the Program Advisory Committee (proposals 2018S2-004) at the Institute of Materials Structure Science, KEK.
Funding Information:
The authors are very grateful to Y. Kuramoto, Y. Matsumoto, and A. Fujimori for their useful discussions and acknowledge A. Wada, N. Hasegawa, D. K. Nguyen, X. Cheng, and E. Sakai for their support in the experiment at PF. This work was financially supported by a Grant-in-Aid for Scientific Research (Nos. 16H02115, 16KK0107, 19H01830, and 20KK0117) from the Japan Society for the Promotion of Science (JSPS), CREST (JPMJCR18T1) from the Japan Science and Technology Agency (JST), and the MEXT Element Strategy Initiative to Form Core Research Center (JPMXP0112101001). A.F.S.-S.
Publisher Copyright:
© 2021, The Author(s).
PY - 2021/12
Y1 - 2021/12
N2 - The metal-insulator transition (MIT), a fascinating phenomenon occurring in some strongly correlated materials, is of central interest in modern condensed-matter physics. Controlling the MIT by external stimuli is a key technological goal for applications in future electronic devices. However, the standard control by means of the field effect, which works extremely well for semiconductor transistors, faces severe difficulties when applied to the MIT. Hence, a radically different approach is needed. Here, we report an MIT induced by resonant tunneling (RT) in double quantum well (QW) structures of strongly correlated oxides. In our structures, two layers of the strongly correlated conductive oxide SrVO3 (SVO) sandwich a barrier layer of the band insulator SrTiO3. The top QW is a marginal Mott-insulating SVO layer, while the bottom QW is a metallic SVO layer. Angle-resolved photoemission spectroscopy experiments reveal that the top QW layer becomes metallized when the thickness of the tunneling barrier layer is reduced. An analysis based on band structure calculations indicates that RT between the quantized states of the double QW induces the MIT. Our work opens avenues for realizing the Mott-transistor based on the wave-function engineering of strongly correlated electrons.
AB - The metal-insulator transition (MIT), a fascinating phenomenon occurring in some strongly correlated materials, is of central interest in modern condensed-matter physics. Controlling the MIT by external stimuli is a key technological goal for applications in future electronic devices. However, the standard control by means of the field effect, which works extremely well for semiconductor transistors, faces severe difficulties when applied to the MIT. Hence, a radically different approach is needed. Here, we report an MIT induced by resonant tunneling (RT) in double quantum well (QW) structures of strongly correlated oxides. In our structures, two layers of the strongly correlated conductive oxide SrVO3 (SVO) sandwich a barrier layer of the band insulator SrTiO3. The top QW is a marginal Mott-insulating SVO layer, while the bottom QW is a metallic SVO layer. Angle-resolved photoemission spectroscopy experiments reveal that the top QW layer becomes metallized when the thickness of the tunneling barrier layer is reduced. An analysis based on band structure calculations indicates that RT between the quantized states of the double QW induces the MIT. Our work opens avenues for realizing the Mott-transistor based on the wave-function engineering of strongly correlated electrons.
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U2 - 10.1038/s41467-021-27327-z
DO - 10.1038/s41467-021-27327-z
M3 - Article
C2 - 34862386
AN - SCOPUS:85120917413
SN - 2041-1723
VL - 12
JO - Nature Communications
JF - Nature Communications
IS - 1
M1 - 7070
ER -