Selective catalytic reduction of N2O with light alkanes over different Fe-zeolite catalysts

S. Kameoka; S. Tanaka; K. Kita; T. Nobukawa; S. Ito; T. Miyadera; K. Kunimori

doi:10.1016/S0167-2991(01)81732-8

Selective catalytic reduction of N₂O with light alkanes over different Fe-zeolite catalysts

S. Kameoka, S. Tanaka, K. Kita, T. Nobukawa, S. Ito, T. Miyadera, K. Kunimori

IMRAM - Division of Inorganic Material Research

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

2 Citations (Scopus)

Abstract

Fe ion-exchanged zeolite catalysts, where Fe-BEA was the most active, were used in the SCR of N₂O with light alkanes (i.e., CH₄, C₂H₆, and C₃H₈) even in the presence of excess oxygen. CH₄ reacted selectively with N₂O even in the presence of excess O₂ (> 250°C: 4N₂O + CH₄ → 4N₂ + CO₂ + 2H₂O), while the reaction of C₂H₆ and C₃H₈ with O₂ was significantly enhanced by the presence of N₂O. N₂O played an important role in the activation of alkanes at an initial step. A mechanism in the SCR of N₂O with light alkanes over Fe-BEA catalyst is proposed. This is an abstract of a paper presented at the 13^th International Zeolite Conference (Montpellier, France 7/8-13/2001).

Original language	English
Title of host publication	Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001
Editors	F. Fajula, F. Di Renzo, A. Galarneau, J. Vedrine
Publisher	Elsevier Inc.
Pages	321
Number of pages	1
ISBN (Print)	9780444502384
DOIs	https://doi.org/10.1016/S0167-2991(01)81732-8
Publication status	Published - 2001
Event	Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001 - Montpellier, France Duration: 2001 Jun 8 → 2001 Jun 13

Publication series

Name	Studies in Surface Science and Catalysis
Volume	135
ISSN (Print)	0167-2991

Conference

Conference	Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001
Country/Territory	France
City	Montpellier
Period	01/6/8 → 01/6/13

Access to Document

10.1016/S0167-2991(01)81732-8

Cite this

Kameoka, S., Tanaka, S., Kita, K., Nobukawa, T., Ito, S., Miyadera, T., & Kunimori, K. (2001). Selective catalytic reduction of N₂O with light alkanes over different Fe-zeolite catalysts. In F. Fajula, F. Di Renzo, A. Galarneau, & J. Vedrine (Eds.), Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001 (pp. 321). (Studies in Surface Science and Catalysis; Vol. 135). Elsevier Inc.. https://doi.org/10.1016/S0167-2991(01)81732-8

Kameoka, S. ; Tanaka, S. ; Kita, K. et al. / Selective catalytic reduction of N₂O with light alkanes over different Fe-zeolite catalysts. Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001. editor / F. Fajula ; F. Di Renzo ; A. Galarneau ; J. Vedrine. Elsevier Inc., 2001. pp. 321 (Studies in Surface Science and Catalysis).

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title = "Selective catalytic reduction of N2O with light alkanes over different Fe-zeolite catalysts",

abstract = "Fe ion-exchanged zeolite catalysts, where Fe-BEA was the most active, were used in the SCR of N2O with light alkanes (i.e., CH4, C2H6, and C3H8) even in the presence of excess oxygen. CH4 reacted selectively with N2O even in the presence of excess O2 (> 250°C: 4N2O + CH4 → 4N2 + CO2 + 2H2O), while the reaction of C2H6 and C3H8 with O2 was significantly enhanced by the presence of N2O. N2O played an important role in the activation of alkanes at an initial step. A mechanism in the SCR of N2O with light alkanes over Fe-BEA catalyst is proposed. This is an abstract of a paper presented at the 13th International Zeolite Conference (Montpellier, France 7/8-13/2001).",

author = "S. Kameoka and S. Tanaka and K. Kita and T. Nobukawa and S. Ito and T. Miyadera and K. Kunimori",

year = "2001",

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editor = "F. Fajula and {Di Renzo}, F. and A. Galarneau and J. Vedrine",

booktitle = "Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001",

address = "United States",

note = "Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001 ; Conference date: 08-06-2001 Through 13-06-2001",

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Kameoka, S, Tanaka, S, Kita, K, Nobukawa, T, Ito, S, Miyadera, T & Kunimori, K 2001, Selective catalytic reduction of N₂O with light alkanes over different Fe-zeolite catalysts. in F Fajula, F Di Renzo, A Galarneau & J Vedrine (eds), Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001. Studies in Surface Science and Catalysis, vol. 135, Elsevier Inc., pp. 321, Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001, Montpellier, France, 01/6/8. https://doi.org/10.1016/S0167-2991(01)81732-8

Selective catalytic reduction of N₂O with light alkanes over different Fe-zeolite catalysts. / Kameoka, S.; Tanaka, S.; Kita, K. et al.
Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001. ed. / F. Fajula; F. Di Renzo; A. Galarneau; J. Vedrine. Elsevier Inc., 2001. p. 321 (Studies in Surface Science and Catalysis; Vol. 135).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Selective catalytic reduction of N2O with light alkanes over different Fe-zeolite catalysts

AU - Kameoka, S.

AU - Tanaka, S.

AU - Kita, K.

AU - Nobukawa, T.

AU - Ito, S.

AU - Miyadera, T.

AU - Kunimori, K.

PY - 2001

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N2 - Fe ion-exchanged zeolite catalysts, where Fe-BEA was the most active, were used in the SCR of N2O with light alkanes (i.e., CH4, C2H6, and C3H8) even in the presence of excess oxygen. CH4 reacted selectively with N2O even in the presence of excess O2 (> 250°C: 4N2O + CH4 → 4N2 + CO2 + 2H2O), while the reaction of C2H6 and C3H8 with O2 was significantly enhanced by the presence of N2O. N2O played an important role in the activation of alkanes at an initial step. A mechanism in the SCR of N2O with light alkanes over Fe-BEA catalyst is proposed. This is an abstract of a paper presented at the 13th International Zeolite Conference (Montpellier, France 7/8-13/2001).

AB - Fe ion-exchanged zeolite catalysts, where Fe-BEA was the most active, were used in the SCR of N2O with light alkanes (i.e., CH4, C2H6, and C3H8) even in the presence of excess oxygen. CH4 reacted selectively with N2O even in the presence of excess O2 (> 250°C: 4N2O + CH4 → 4N2 + CO2 + 2H2O), while the reaction of C2H6 and C3H8 with O2 was significantly enhanced by the presence of N2O. N2O played an important role in the activation of alkanes at an initial step. A mechanism in the SCR of N2O with light alkanes over Fe-BEA catalyst is proposed. This is an abstract of a paper presented at the 13th International Zeolite Conference (Montpellier, France 7/8-13/2001).

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U2 - 10.1016/S0167-2991(01)81732-8

DO - 10.1016/S0167-2991(01)81732-8

M3 - Conference contribution

AN - SCOPUS:84981709219

SN - 9780444502384

T3 - Studies in Surface Science and Catalysis

SP - 321

BT - Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001

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A2 - Di Renzo, F.

A2 - Galarneau, A.

A2 - Vedrine, J.

PB - Elsevier Inc.

T2 - Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001

Y2 - 8 June 2001 through 13 June 2001

ER -

Kameoka S, Tanaka S, Kita K, Nobukawa T, Ito S, Miyadera T et al. Selective catalytic reduction of N₂O with light alkanes over different Fe-zeolite catalysts. In Fajula F, Di Renzo F, Galarneau A, Vedrine J, editors, Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001. Elsevier Inc. 2001. p. 321. (Studies in Surface Science and Catalysis). doi: 10.1016/S0167-2991(01)81732-8