Clear difference between the chemical structure of SiO2/Si interfaces formed using oxygen radicals versus oxygen molecules

Tomoyuki Suwa, Yuki Kumagai, Akinobu Teramoto, Takayuki Muro, Toyohiko Kinoshita, Tadahiro Ohmi, Takeo Hattori

研究成果: Conference contribution

1 被引用数 (Scopus)

抄録

Soft-x-ray-excited angle-resolved photoelectron spectroscopy studies on silicon dioxide films formed using oxygen radicals (OR) versus oxygen molecules (OM) are reported. Most of intermediate oxidation states of Si, so called suboxides, consisting of Si3+, Si2+, and Si1+ are localized at and near the SiO2/Si interfaces. The suboxides formed utilizing OM are located extremely close to the interfaces, while suboxides formed utilizing OR are located not only at the interface but also in the Si substrate. This implies the penetration of a part of OR into the Si substrate to form Si1+ and to relax the interfacial stress. Intermediate chemical bonding states of Si are formed in Si substrate closer to the interface as compared with those formed utilizing OM. This implies that the interfacial stress in the former is smaller than that in the latter.

本文言語English
ホスト出版物のタイトルSilicon Nitride, Silicon Dioxide, and Emerging Dielectrics 11
出版社Electrochemical Society Inc.
ページ115-122
ページ数8
4
ISBN(電子版)9781607682158
ISBN(印刷版)9781566778657
DOI
出版ステータスPublished - 2011

出版物シリーズ

名前ECS Transactions
番号4
35
ISSN(印刷版)1938-5862
ISSN(電子版)1938-6737

ASJC Scopus subject areas

  • 工学(全般)

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