Potential energy of hydrogen atom motion on Pd(111) surface and in subsurface: A first principles calculation

Nobuki Ozawa, Tanglaw A. Roman, Hiroshi Nakanishi, Hideaki Kasai, Nelson B. Arboleda, Wilson Agerico Diñ

研究成果: Article査読

50 被引用数 (Scopus)

抄録

We calculate the adiabatic potential energy for hydrogen atom motion on a Pd(111) surface and in a subsurface within the framework of the density functional theory in order to understand the diffusion mechanism of a hydrogen atom from the Pd(111) surface to the subsurface. According to the calculated adiabatic potential energy surface for the hydrogen atom motion up to the third atom layer, an effective diffusion path of the hydrogen atom into the Pd bulk starts from the fcc hollow site on the Pd(111) surface. Moreover, the diffusion path passes through the octahedral site between the first and the second Pd atom layers, the tetrahedral site beneath a Pd atom of the first layer or above the Pd atom of the third layer, and the octahedral site between the second and third layer.

本文言語English
論文番号123530
ジャーナルJournal of Applied Physics
101
12
DOI
出版ステータスPublished - 2007
外部発表はい

ASJC Scopus subject areas

  • 物理学および天文学(全般)

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